Next, work on the shortbread crust. Preheat the oven to 350°F / 175°C. Spray 3, 8-inch cake pans with nonstick spray, then line with parchment rounds.
Use a fork or pastry cutter to combine 1 1/2 cups softened butter, 3 cups flour, 3/4 cup powdered sugar, and 1 tsp fine salt. It should form a slightly crumbly dough once combined.
Divide the dough into three equal portions and press them into the bottom of the prepared pans with your fingers to create an even layer.
Prick the crust thoroughly with a fork, then bake for 22-25 minutes, or until the edges are just starting to brown. Place the pan on a wire rack to cool and keep the oven.
Chocolate Cake Layers
Sift or whisk together 2 1/2 cups flour, 2 1/2 cups sugar, 1 cup cocoa powder, 2 1/2 tsp baking powder, 2 tsp baking soda, and 1 tsp salt into a large bowl.
Add 1 1/4 cups warm water, 1 1/4 cups buttermilk, 2/3 cup oil, 3 eggs, and 2 tsp vanilla into a separate large bowl and whisk together until combined.
Mix the dry ingredients into the wet ingredients until they're incorporated, and the batter is smooth.
Pour the batter evenly between the prepared pans on top of the baked shortbread crusts. Bake for about 28-32 minutes in the preheated 350 F / 175 C or until a toothpick comes out with a few moist crumbs.
Remove the cake layers from the oven and let them cool in the pans for about 10 minutes. Gently run an offset spatula around the rim of the cake pans to loosen them, then carefully flip them into wire racks to finish cooling. Leave the parchment rounds underneath each crust to help keep it intact.
Once cooled, use a serrated knife to level the top of each cake layer. If you are making these cake layers in advance, wrap and freeze them at this point. These can be made up to a month in advance.